SCI论文写作重要结构2

1. Opening up enormousopportunities to prepare high performance rubber

composites for future engineering applications.

2. In order to tackle this global issue, new oil-independent fillers have

received increasing attentions for replacement of CB.

3. (溶液混胶) However, conventional mechanical blending method cannot

uniformly disperse the GO sheets inthe rubber matrix (see Supplementary Information S10). Solution mixing12–15 has been demonstrated to be aneffective way to obtain the desired dispersion, but the removal of organic solvents poses persistent problems suchas added cost and potential environmental pollution for the practical implementation of the method.

4. The GO/SBR composites formed by this route exhibit

unprecedentedreinforcing efficiency of GO towards SBR

5. The GO dispersion in composite and the interface interaction are thetwo

main factors to determine the reinforcing efficiency of GO in thecomposite.

6. Moreover, any eventual replacement of CB by GO will

haveepoch-making significance（划时代的）in the oil-dependent rubber industry.

7. As shown in Fig. 4e, the storage modulus of theSBR/GO composite

increases with the GO content increasing,throughout the range of temperatures investigated, indicating thatthe elastic response of neat SBR towards deformation is stronglyinfluenced by the presence of nanodispersed GO sheets.

8. Carbon nanotubes (CNTs) have attracted great research interestsince

their discovery in 1991 by Iijima [1] due to their unique properties which include: chemical stability, excellent mechanicalstrength, high surface area and extraordinary high electrical conductivity [2,3].

9. The substrate’sgeometry effect on the catalyst distribution and on the

characteristics of the synthesized nanotubes has not been exhaustively stated.

10. However,until now, research on the mechanical and thermal

properties ofepoxy resin filled with graphene-based hybrid fillers is scarce.（缺乏的）

11. Metallic fillerssuffer the disadvantage of high density，What's worse,

metallicfillers

usually

deteriorate

the

strength

of

rubber

material.Forceramic fillers and carbon nanotubes, the high price is a bottle neckto their extensive application [11]. Thus, it is of great academic andindustrial interests to develop fillers with high thermal conductivity, low density, excellent reinforcement performance as well asa reasonable cost.

12. However, the presence ofbulk rubber chains could form “protective

layers” around the GOsheets, giving rise to(导致) partial reduction GO

13.

（溶液混胶后上辊）The addition of the curing agents was carriedout in

an LN-120 open two-roll mill (LINA machinery Industrial Co.Ltd., China) at room temperature.

14. Guo et al. [39] reported that GO couldbe reduced to single layer GE

successfully in the presence of PVPand formed a stable dispersion in water, which offers a goodinspiration（启发） for the fabrication of RGO/rubber nanocomposite bylatex heterocoagulation

15. And their synergistic effect in enhancing the properties of poly(vinyl

alcohol) (PVA) nanocompositeswas investigated.

16. This synergistic effect improved the dispersion homogeneity by

avoiding the agglomeration phenomenon of nanofillers within the polymer matrix, resultingin nanocomposites with largely enhanced properties compared to those prepared from single nanofiller(CNC or GON).

17. Recently, hybrid reinforcements of polymer nanocomposites are

gaining increased acceptance.

18. in order to understand the synergisticeffect generated from the

combination of both kinds of nanomaterials, three C:G hybrid nanofillers have been prepared by varyingtheir weight ratio (i.e. C:G-2:1, C:G-1:1 and C:G-1:2).

19. The samples were coded as(标记为) C:G-2:1, C:G-1:1 and C:G-1:2

for C:G hybrids at mass ratio of 2:1, 1:1 and 1:2,respectively.

20. Recently, a variety of promising materials serving as

anti-g-raycoating and the mechanisms of the irradiation on the materialshave been proposed

21. Multiple assays（多种表征） were employed to introduce the

chemicalstructure of graphene oxide.

22. Acetic acid wasadopted to adjust pH, the pH value is buffered （缓冲）

closed to 3.5.

23. After storage for several weeks, the dispersion of FGO still remains

stable while GO forms a precipitate.

24. ESR (see Fig. 5(a)) was performed to ascertain

（确定）the

influence ofthe irradiation on the oxidation index

25. Recently, graphene and carbon nanotube (CNT) composites have

attracted great interest of scientists andexhibited fascinating properties even better than they could on their own

26. The CNTs had several tens of micrometers in length and 50–200 in

diameter.

27. Among them, nanotubes and grapheneare the most dazzlingstars in

the field of nanotechnology.

28. Compared toCNTs, graphene, a two-dimensional (2D) hexagonally

atomic carbon film, also possesses the above mentioned properties of CNTsas well as its special features, e.g., high light transmittance [8]and high reactivity of graphene edges [9], and has shown greatcharm in nanocarbon family.

29. A home-made nickel case, ? 50 mm (diameter) 10 mm(height) 20lm

(thickness), was cleaned by sequence processwith ethanol, acetone, and distilled water for 10 min.

30. These results indicate that the pressure playsa decisive role to

synthesize the fiber-like nanocarbons includingCNTs and g-CNTs in MPI process.

31. This is not only that valorizing waste biomass to achievehigh-value

nanocarbons, but also that solving the environmentnuisance（损害） caused by the huge quantity of waste biomass。

32. Other advantages of sulfur includenatural abundance, low cost and

environmental benignity, makingit an attractive choice as cathode material for next-generation energy storage devices.

33. These films were denoted as 1GO/5CNT, 1GO/2CNT and 1GO/

1CNT interlayers.

34. The elemental mapping of interlayersafter cycles was carried out on

an energy dispersive spectrometer(EDS) linked to SEM 6390.

35. Physical and chemical vapor deposition methods to synthesizethin

films are also described quite often but all of them aredogged by （受困

于）the elimination of the very stable N2, which results indisordered,

quite carbon-rich materials.

36. Thermoanalyticalmethods (TGA, DSC) in combination with

XRD were used to characterize the intermediate steps along the condensation of the molecular precursor.

37. However, the principal difference between the graphene and

MWCNT lies in their shapes. Graphene has a plate-likeshape and is bi-dimensional, whereas MWCNTs are uni-dimensional with high aspect ratio.

38. In the second stage thecuratives(橡胶小料) were added to rubber

compound using a two-roll mill.

39. The DC electrical resistivities of the rubber compounds are plottedin

Fig. 3 as function of filler loading.

40. The 5 phr EG filled compound showed a mostlyagglomerated

structure, whereas GnP showed a wrinkled paperlike morphology of the GnP.

41. The electroless plating improved the mutual disperse of GNPs and

the Cu matrix

42. Benefiting from better dispersion and stronger interfacial bonding,

the increase of 64.5% in yield strengthwas obtained in the 0.5% Ni-GNPs/Cu composite.

43. After that, the products were washedwith ethanol thoroughly.

44. However, BMI resin suffers from inherent brittleness becauseof its

highly cross-linked structures, and some micro-cracks areeasily generated and propagated under friction stress [5], whichgreatly hinders practical application of BMI resin as wear-resistantmaterials in many fields.

45. The incorporation of nanoparticles with RGOsheets in the

composites can not only prevent the aggregation ofgraphene and nanoparticles but also promote them produce synergetic effects.

46. Therefore, it is highly preferred to have the graphene

orienteduniformly throughout the bulk of the composites, which will makegood use of the in-plane self-lubrication of grapheme.

47. The reduced graphene oxide (RGO) wasalso prepared in similar

procedures in the absence of Fe3O4 toperform a contrast experiment

48. Unfortunately, the impact strength of the composites declines when

theamount of fillers is further increased, which is due to the fact thatexcessive fillers can not be well dispersed in the BMI matrix andagglomerate to cluster.

49. Fig. 5a represents the fracture surface of neat BMI resin, a

relativelysmooth surface with occasional river patterns, which exhibits atypical brittle feature.

50. These stronginterfacial interactions enable graphene to bring its

amazing mechanical properties into resin matrix, achieving a perfect

reinforcing and toughening material.

51. In some circumstances, wear resistance of materials is an extremely

importantevaluation index which directly determines service life of products

52. Weinvestigated the essential factors and mechanisms responsible

forthe observed mechanical and tribological properties and attempted to

determine

the

relationship

between

mechanical

and

tribologicalproperties.

53. As themass fraction of the fillers is above 0.8 wt%, the hardness of

BMIcomposites slowly increases with the increasing of the filler contents.

54. The BNNSs/NR nanocomposite was further processed by strong

shearing on a two-rollmill, as was the BNNSs/SiR composite.

55. Nevertheless, the commercialization ofLieS batteries has been

severely limited by several issues.

56. Extensive studies have been carried out to alleviate the aboveissues,

focusing mainly on developing novel cathode materials.

57. Scientists are trying hard to increase both thecapacity and stability in

the whole long cycling process.

58. Such an unparalleled(无与伦比的) structure of SnO2@3DG would

beexpected to have superior performance for lithium storage.

59. Fig 2D presents a typical HRTEM image of ananoparticle in dark,

contrast in Fig. 2B. It clearly exhibited the lattice fringes with a d spacing of 0.203nm, corresponding to the interplanar distance of(110) planes of metallic Fe. Energy dispersive X-rayspectroscopy (EDS)

measurements also e videncedthe existence of element iron and nitrogen (Fig. 2E).The signal of element copper in Fig. 2E should befrom copper grid used for TEM observation.

60. The design idea described here could be extended to synthesize

other similar catalysts in acost-effective and scalable way for wide applications.

61. However, Pd is a precious noble metal whose high cost impedes（阻

碍）the commercialization of DAFCs.

62. In general, the catalytic activity of metal catalysts for the alcohols

oxidation reaction strongly depends on the nature ofCNTs support in terms of the surface area, conductivity, andchemical properties.

63. In their study, DMFC performanceof PtRu catalyst decreased in

the order ofcarbonsupport:graphitic

carbon nanofiber

(GCNF)>SWNTs>MWNTs.

64. The number of walls and outer diameter of CNTs were taken as

average over more than ten TEMimages for each CNTs sample.

65. (用拉曼表征碳管)CNTs were examined by Raman spectroscopy at

room temperature with excited laser wavelength and power density of1064 nm￠1 and 5 mWcm￠2, respectively (Figure 1A). The Dband in 1281 cm￠1 derives from the amorphous carbon anddefects, while the G band in 1589 cm￠1 indicates the graphitelayer of CNTs.[22] The intensity ratio of defect-derived D band(ID) to graphite-derived G band (IG) reflects destructiveness ofthe SP2 hybridized carbon atom. Thus, the increase of theID/IG ratio is an indication of the destructiveness or the defectformation of the CNTs surface.

66. （XRD说法）The crystallinenature of Pd NPs was confirmed

by XRD (Figure S3, SupportingInformation). The peak at 25.98 is attributed to the hexagonalcarbon structure of CNTs in (002) plane.[32] The 2q values of40.08 correspond to the diffraction peaks of Pd (111) with dspacing of 0.23 nm, while 2q value of 46.38, 67.88, and 80.68correspond to Pd (200), Pd (220), and Pd (311), respectively.

67. In addition, the Pd (311) diffraction peak for Pd-CNTs-1 and

Pd-CNTs-2is discernible but of much low intensity, which may be due tothe fact that···········

68. Pd NPs with controlled particle size have been uniformly assembled

and anchored on the surface of CNTs .

69. Although improved cell performancewas achieved, the methods

used in preparing these compositematerials generally involve complex, multi-step synthetic processes. In addition, the severe self-discharge of LieS batteriesinduced by polysulfides has not been fully solved.

70. The unique structural features of PAN/GO nanofiber separatorcan

play an important role in improving the overall performance ofLieS cells.

71. Fumed alumina is inferior to（劣于）organobentonite for increasing the

toughness or longitudinal compressive modulus

72. Supercapacitors (SCs), also called electrochemical capacitors(ECs),

have gained substantial amount of attention for their excellent power density (1~2 orders of magnitude higher than batteries),long cycle stability (2~3 orders of magnitude larger than that ofbatteries), and

relatively high energy density (almost 3~4 orders ofmagnitude larger than conventional capacitors)

73. Recently, iron oxyhydroxide (FeOOH) is considered to be

apromising anode material in terms of its unique open twodimensional (2D) layered structure, low cost, natural abundanceand environmentally friendly

74. Graphene oxide (GO) solution was firstly prepared by theoxidation

of natural graphite powders based on a modified Hummer's method.

75. However, thefacile stacking nature induced by the strong p-p

interaction andvan der Waals forces between graphene layers hinders the fulldemonstration of intrinsic properties of grapheme.

76. Such DTG affords impressive properties in the field of

supercapacitors, batteries, and electrocatalysis.

77. In most cases, the edges of the graphenenanosheets arealways

saturated with an abundance of oxygen-containing functional groups.

78. The composition of the graphene sample was also validatedthrough

the gravimetric elemental analysis.

79. The uniformdispersion of GNS-Fe3O4@PZM in BMI matrix will

prompt theexcellent properties of graphene to be fully used.

80. urthermore, this study may open a new route foroptimizing interface

structure

and

improving

the

comprehensiveproperties

of

graphene-polymer composites.

81. Recently, researches on GO sheets haveprogressed remarkably in a

wide variety of applications by LBL selfassembly technique, such as enhancement in mechanical property, super electrical devices like

battery and super capacitors, and gas barrier application .

82. Fig. 10 shows the TGA curves of (PEI/XNBR/PEI/GO)30 film and

XNBR latex film, which are employed to search for the thermalbehavior difference between pure XNBR latex film and LBL film.

83. It hasattracted a lot of considerable theoretical and experimental

researches, mainly related to the remarkably essential properties, such as the ultrahigh carrier mobility, [4] superior thermalconductivity, [5] and quite large tensile strength, [6] and so on.

84. Because of their high aspect ratio,carbon nanotubes are superior

solution to the other fillers and havebeen used by many researchers to improve the conductivity ofinherently insulating polymers.

85. Excellent properties combined with strong strength, high modulus,

light weight, superior chemical resistance and outstandingthermal stability make CFs reinforced advance polymer compositesideal structural materials to be used widely in the automotive andaerospace industries

86. Obviousdistinctions in surface morphologies between untreated and

modified CFs can be observed.

87. The enhancement of surfaceroughness can improve obviously the

interfacial propertiesthrough providing more contact points and increasing mechanicalinterlocking between CFs and MPSR matrix.

88. A special emphasiswas also placed on studying the film formation

mechanismsbetween acrylate and rGO sheet to further elucidate the reasonsbehind the outstanding properties of P2EHA/NH2-rGO

composites.

89. Thisstrategy can be anticipated to provide a platform to prepare

polymer/graphene

composites

with

high

performance

and

multifunctionality for potential application in various areas.

90. There are a very negligible trace of water in the composites,

confirming the complete evaporation of moisture due to curing at a high temperature.

91. Another interesting finding from Fig. 11(a) and (b) was that the

conductivities of the composites along the alignment direction and that perpendicular to it revealing a remarkable difference between the two direction as the result of the anisotropic, aligned structure.

92. GO is a layeredmaterial featuring a variety of oxygen-containing

functionalitieswith epoxide and hydroxyl groups on the basal plane and carbonyland carboxyl groups along the edges.

93. Lin et al. found that large-size graphemeoxide (GO) sheets can

impart a tremendous positive impact onself-alignment of graphene papers.

94. To address the deficiencies of poor electronic conductivity and

strong tendency towards aggregationsuffered by V2O5 nanosheets, here we propose a facile and elegant self-organization strategy todecorate them simultaneously with Ag nanoparticles and TiO2 nanorods, resulting in novel twodimensional hybrid architectures.

95. The resulting two-dimensional hybrid architectures exhibit

synergistic superiorities in reversible capacity,rate capability and cycle stability over neat V2O5 nanosheets, and hold great promise as a

cathodematerial of lithium-ion batteries

96. Because of this shortcoming, researching alternativecathode

materials with higher reversible capacity, rate capability and cycle stability is of vital importance.

97. Filler size and segregation, as observed by scanning electron

microscopy, play important roles in determining the electrical properties of silicone elastomer filled composites.

98. Different filler dimensions have diverse effects onthe composite

properties.

99. The arrow in Figure 1(c) indicates that CB particles are separated

from each other.This fact is one of the reasons that the electrical resistivity did not decrease.

100. Amine functionalized CNT were addedto the epoxy resin to generate

covalent bonding with thepolymer matrix

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